STRUCTURAL HIERARCHIES IN INORGANIC SYSTEMS

Hierarchical structure is most obvious in organic and higher systems . Cyril Stanley Smith discussed hierarchical order in inorganic systems. In a historical note he said that one of the most surprising results from applying x-ray diffraction to the study of crystals in 1912 was that:

Most inorganic solids contain no molecules, or rather that the whole crystal is the molecule, In sodium chloride, for instance, there is no specific pairing of sodium and chlorine atoms any more than there is in solution; the atomic ratios called for by that masterly summary of Daltonian principles, the law of simple combining proportions, are in most cases due to the exigencies of charge and the geometric limitations imposed by the crystal lattice, not to the formation of molecules.

Since that time, our knowledge of crystaline structure has increased greatly and with it a new vision of crystals has emerged. In a typical crystal, he explained, "The outlines of the crystal grains are more reminiscent of the froth on a glass of beer than of geometric polyhedra." He went on to explain why that is:

Here it should be noted that a single individual, whether an atom, a crystal, or anything else, can take whatever shape is natural to it, but in an aggregate, the individuals each share an interface with another one in a zone of mutual conformity. Moreover, unless some action occurs across this interface which results in an internal change in the structure of both of the contacting units there is no basis for structural aggregation. Although atoms may appear as "hard and shinly balls" when viewed on a large enough scale, they attract each other only because they possess an internal structure that is directly influenced by their external environment. This interaction between inside and outside as seen by an individual is the very basis of a hierarchy of any kind whatever.

Grain boundary is not recognizable in groups of a few atoms. It is the property only of an aggregate large enough for divergent group properties to emerge. In any sufficiently large array there will be areas of local departure from order (due to entropy or to the randomness of its history), At a high scale of resolution the boundaries are fuzzy, their existence a question of definition involving connections beyond the normal field of the viewer. At a lower magnification the boundaries will appear sharp and distinct, at still lower magnification they disappear again. Smith continued:

In systems of any kind, change depends on the formation and/or movement of interfaces. A polycrystalline aggregation can arise in a thermodynamically unstable environment from either the discontinuous nucleation of new crystals and the enlargement of these until they impinge upon each other, or from the gradual condensation of imperfections to leave more perfect regions.

The former change is a first order or high energy change, the second, a relatively low energy change. The result, however, may be indistinguishable since the process ends by the boundaries adjusting to their own needs. Smith gave two examples: In a pure metal the first corresponds to the growth of crystals from the liquid or from another (unstable) crystalline form, the latter to the recovery of a cold-worked material, in which the imperfections (dislocations and vacancies) which are at first widely scattered throughout the volume of the strained crystal collect together to form a network of sub-grain boundaries. The sub-grain boundaries themselves may further condense, but often they are swept away by the movement through them of the major boundaries (recrystallization)--a process that on a large scale appears as a nucleation and growth process. In most cases when the grains have reached composition equilibrium throughout their volumes, further geometric change occurs simply by movements of the grain to decrease their area and hence the energy of the system.

He proposed several principles of the hierarchies that deal particularly with inorganic structure.
The world is complex and understanding is simple; however,.there is always some scale on which significant interaction involves relatively few units.. The newú structures that seem to emerge as aggregates on a larger scale are partly illusory: It is less of a characteristic of the structure itself than of the limited resolution of our perception (whether visual or conceptual). Each level is what we see at certain resolutions, and corresponds to the matching of only those structural elements that can be resolved without too much detail at a single effect viewing distance.

1. An assembly of units will not form a coherent aggregate unless the parts interact in such a way as to modify their internal structure and energy. An organism is an aggregate in which there is a dominant center of organization and significant internal communication. (A physically unconnected assembly can be related intellectually as a structure in the mind of an observer.)

2, An aggregate that is neither completely ordered nor completely disordered must have hierarchical aspects, but the perception of the levels of the hierarchy requires the recognition of a two-dimensional surface to define each three-dimensional unit according to Euhler's law. In general, the surface is defined by interactions between discontinuities of the coordination of the parts on the next lower level; discontinuities not so connectable constitute merely internal features. The number of imperfections, and hence the number of possible interfaces, increases with size for simple reasons of entropy.

3 Each scale of structure has a type and energy of interaction appropriate to it. Structure and energy are inseparable. Though the strongest interactions between any units are those between neighbors on the same scale, residual effects extend downwards for a fewú and upwards through many levels--but not indefinitely, for beyond a certain point complexity becomes irresolvable and merges again with homogeneity. A human being is not far from the point of maximum significant complexity that can be usefully associated with quantum interaction between chemical atoms, while the planets and their satellites are not far from the smallest gravitationally-determined structures.

4. Complex structures cannot originate instantaneously but are formed in time; they must have a, history. A complex structure is both a partial record of past history and a framework within which future changes occur by the operation of physical laws.

5. Structural change occurs by the formation of interfaces and/or by their movement. New interfaces can form internally by the progressive condensations of imperfections causing the self-enhancements of fluctuations until the gradients are sharp enough to become definable interfaces, The external growth of an individual unit occurs by acretion wúhich causes the translation of an existing interface. The latter is typical of crystal growth, the former of spinodal transformation, biological cell division, convection cells and stream-bed formation.

6, A complex aggrúegate may contain superimposed several different structural hierarchies (each corresponding to a different type of interaction between units, based on different aspects of internal strvcture). The hierarchies may be partially independent or their various levels may interfere constructively or destructively with each other. In organic aggregates all interactions, not necessarily those between adjacent atoms, are those quantized photons transmitting electrical or magnetic fields, In biological organisms there are superimposed more complex interactions based on mass transfer of chemical messengers wúhich react only wúith specific complex local arrangements; in intellectual or social systems small and large thought patterns interlock and new patterns arise in the constructive mismatching of communicated parts of the old.

In conclusion Smith stated that historically it was the artists who discovered the symmetries that arise in the repetition of identical motifs regardless of their shape. They have a greater sense of the relationship of parts to wholes than most scientists, "Perhaps the scientists concern with accuracy of statements, which by its very nature must be limited, needs to be tempered a little more than it has been in recent years with the artists awareness of larger scale interactions,"

Self-Similar Hierarchical Order

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